Hi,
VinylStudio cannot do this currently, but you are not the first person to ask and it is on our to do list. In the meantime, there is a simple way to achieve what you want. Make your recordings in a 'throw away' collection on the laptop, then create the albums again on the desktop and import the recordings made on the laptop (I assume the machines are networked together). When you import a recording, use the 'Copy file to VinylStudio's recordings folder' option and this will copy the file across automatically. You can then delete the album on the laptop to save disk space. This all takes longer to describe than it actually takes to do and there is no need to create a new collection on the laptop for each album you record.
The next version of VinylStudio will make this task a little easier by offering to record all sides of an album as a single file. You will have to import each side separately, currently.
Hope this helps. Another of our users is doing something similar and it works for him.